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New Strategies for N-Heterocyclic Carbenes Catalyzed Annulations on Hardback by Xiangyu Chen
New Strategies for N-Heterocyclic Carbenes Catalyzed Annulations on Hardback by Xiangyu Chen
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New Strategies for N-Heterocyclic Carbenes Catalyzed Annulations

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Description

This thesis focuses on NHC-catalyzed annulation of nitroalkenes, enals and α,β-unsaturated carboxylic acids. (1) NHCs were found to be efficient catalysts for the [4+2] annulation of β-substituted nitroalkenes. The scope of Rauhut–Currier reaction was successfully extended to the most challenging β-substituted alkenes by this method; (2) Enals were successfully used for [4+2] annulations with azodicarboxylates catalyzed by NHC via γ-addition. Highly enantiopure tetrahydropyridazinones and γ-amino acid derivatives could be easily prepared by subsequent transformations of the resulting dihydropyridazinones. (4) The readily available α,β-unsaturated carboxylic acids were first successfully employed to generate the α,β-unsaturated acyl azolium intermediates by using NHC for the enantioselective [3+2] and [3+3] annulations.
Release date NZ
December 30th, 2016
Author
Audience
  • Professional & Vocational
Edition
1st ed. 2017
Illustrations
13 Illustrations, color; 53 Illustrations, black and white; XIV, 123 p. 66 illus., 13 illus. in color.
Pages
123
Dimensions
155x235x10
ISBN-13
9789811028984
Product ID
26083709

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